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Double core-hole states in SiX4 (X = F, Cl, Br, and CH3) molecules derived by photoelectron and KLL Auger spectroscopy
Free Univ Berlin, Inst Expt Phys, Berlin, Germany..
CNRS, Lab Chim Phys Mat & Rayonnement, UMR 7614, F-75700 Paris, France.;Univ Paris 06, Univ Paris 04, UMR 7614, LCPMR, F-75252 Paris 05, France..
CNRS, Lab Chim Phys Mat & Rayonnement, UMR 7614, F-75700 Paris, France.;Univ Paris 06, Univ Paris 04, UMR 7614, LCPMR, F-75252 Paris 05, France..
CNRS, Lab Chim Phys Mat & Rayonnement, UMR 7614, F-75700 Paris, France.;Univ Paris 06, Univ Paris 04, UMR 7614, LCPMR, F-75252 Paris 05, France..
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2015 (English)In: Journal of Physics, Conference Series, ISSN 1742-6588, E-ISSN 1742-6596, Vol. 635, 112057Article in journal (Refereed) Published
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Abstract [en]

In recent years double core-hole states are intensively studied since their chemical shifts provide detailed information about initial-state and relaxation effects in a molecule. We derived the Si 1 s(-1), 2s(-1) and 2p(-1) binding energies as well as the Si 2s(-2), 2(p-1)2p(-1), and 2p(-2) double-core hole binding energies of different SiX4 systems in order to derive the chemical shifts. Based on these results we created Wagner plots, which give insight in the initial state and the relaxation effects in the different molecules.

Place, publisher, year, edition, pages
2015. Vol. 635, 112057
National Category
Physical Sciences
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URN: urn:nbn:se:uu:diva-279233DOI: 10.1088/1742-6596/635/11/112057ISI: 000366407000639OAI: oai:DiVA.org:uu-279233DiVA: diva2:907977
Conference
29th International Conference on Photonic, Electronic, and Atomic Collisions (ICPEAC), JUL 22-28, 2015, Toledo, SPAIN
Available from: 2016-03-01 Created: 2016-02-29 Last updated: 2017-11-30Bibliographically approved

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Piancastelli, Maria Novella
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