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Quasi two-step dissociation effects observed in the core excited OCS molecule
KTH, School of Engineering Sciences (SCI), Physics.ORCID iD: 0000-0001-7389-5501
1998 (English)In: Chemical Physics Letters, ISSN 0009-2614, E-ISSN 1873-4448, Vol. 285, 71-76 p.Article in journal (Refereed) Published
Abstract [en]

Studies of the decay dynamics following carbon 1s and sulfur 2p electron excitations of the OCS molecule using the photoelectron–photoion–photoion coincidence method and a synchrotron radiation source are presented. A Monte Carlo code is utilized to interpret the data obtained, which together with previous measurements including branching ratios, kinetic energy distributions and ionic b-parameters give new information on the dynamics of three-body dissociation processes. The results indicate that the instantaneous and sequential dissociation models should be replaced by quasi two-step models.

Place, publisher, year, edition, pages
Elsevier, 1998. Vol. 285, 71-76 p.
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Natural Sciences
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URN: urn:nbn:se:kth:diva-182815OAI: diva2:905838


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Rachlew (Källne), Elisabeth
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