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Increased Cycling Efficiency of Lithium Anodes in Dimethyl Sulfoxide Electrolytes For Use in Li-O-2 Batteries
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Structural Chemistry.ORCID iD: 0000-0003-2538-8104
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Structural Chemistry.
Uppsala University, Disciplinary Domain of Science and Technology, Chemistry, Department of Chemistry - Ångström, Structural Chemistry.
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2014 (English)In: ECS ELECTROCHEM LETT, ISSN 2162-8726, Vol. 3, no 6, A62-A65 p.Article in journal (Refereed) Published
Abstract [en]

High lithium cycling efficiencies are required if a metal anode system is to be considered for use in Li-O-2 batteries. In this work electrolyte additives (0.3 M LiNO3 and 0.14 M VC) were used to increase the efficiency from 25 to 82.5% in the topical DMSO based electrolyte. Furthermore, we show that oxygen also acts to improve the cycling efficiency to 87%. This work highlights the importance of anode considerations in the development of metal O-2 batteries in alternative solvents (DMSO, Acetonitrile and DMA) and suggests realistic strategies for performance improvements. (C)The Author(s) 2014. Published by ECS. This is an open access article distributed under the terms of the Creative Commons Attribution 4.0 License (CC BY, http://creativecommons.org/licenses/by/4.0/), which permits unrestricted reuse of the work in any medium, provided the original work is properly cited. All rights reserved.

Place, publisher, year, edition, pages
2014. Vol. 3, no 6, A62-A65 p.
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Chemical Sciences
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URN: urn:nbn:se:uu:diva-227581DOI: 10.1149/2.007406eelISI: 000336012400007OAI: oai:DiVA.org:uu-227581DiVA: diva2:730457
Available from: 2014-06-27 Created: 2014-06-27 Last updated: 2016-04-26Bibliographically approved

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Younesi, RezaRichardson, WilliamLiu, JiaGustafsson, TorbjornZhu, JiefangEdström, Kristina
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