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Electronic structure of tris(8-hydroxyquinoline) aluminum thin films in the pristine and reduced states
Linköping University, Department of Physics, Chemistry and Biology. Linköping University, The Institute of Technology.
Sumitomo Chem Co Ltd, Japan.
Linköping University, Department of Physics, Chemistry and Biology, Computational Physics. Linköping University, The Institute of Technology.
Linköping University, Department of Physics, Chemistry and Biology, Surface Physics and Chemistry. Linköping University, The Institute of Technology.
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1999 (English)In: Journal of Chemical Physics, ISSN 0021-9606, E-ISSN 1089-7690, Vol. 111, no 5, 2157-2163 p.Article in journal (Refereed) Published
Abstract [en]

The electronic structure of tris(8-hydroxyquinoline) aluminum (Alq(3)) has been studied in the pristine molecular solid state as well as upon interaction (doping) with potassium and lithium. We discuss the results of a joint theoretical and experimental investigation, based on a combination of x-ray and ultraviolet photoelectron spectroscopies with quantum-chemical calculations at the density functional theory level. Upon doping, each electron transferred from an alkali metal atom is stored on one of the three ligands of the Alq(3) molecule, resulting in a new spectral feature (peak) in the valence band that evolves uniformly when going from a doping level of one to three metal atoms per Alq(3) molecule. (C) 1999 American Institute of Physics. [S0021-9606(99)50628-4].

Place, publisher, year, edition, pages
American Institute of Physics (AIP) , 1999. Vol. 111, no 5, 2157-2163 p.
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Engineering and Technology
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URN: urn:nbn:se:liu:diva-81302DOI: 10.1063/1.479486ISI: 000081698700043OAI: oai:DiVA.org:liu-81302DiVA: diva2:551453
Available from: 2012-09-11 Created: 2012-09-11 Last updated: 2017-12-07

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