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Plasmon-Enhanced Optical Control of Magnetism at the Nanoscale via the Inverse Faraday Effect
Swiss Fed Inst Technol, Dept Mat, Lab Mesoscop Syst, CH-8093 Zurich, Switzerland.;Paul Scherrer Inst, Lab Multiscale Mat Expt, CH-5232 Villigen, Switzerland.;European XFEL, Holzkoppel 4, D-22869 Schenefeld, Germany..ORCID iD: 0000-0002-4320-4957
Swiss Fed Inst Technol, Dept Mat, Lab Mesoscop Syst, CH-8093 Zurich, Switzerland.;Paul Scherrer Inst, Lab Multiscale Mat Expt, CH-5232 Villigen, Switzerland.;Paul Scherrer Inst, Lab Nano & Quantum Technol, CH-5232 Villigen, Switzerland..ORCID iD: 0000-0002-1642-4786
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy.ORCID iD: 0000-0001-9555-0619
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Physics.ORCID iD: 0000-0002-6105-1659
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2025 (English)In: ADVANCED PHOTONICS RESEARCH, ISSN 2699-9293, Vol. 6, no 1Article in journal (Refereed) Published
Abstract [en]

The relationship between magnetization and light has been the subject of intensive research for the past century. Herein, the impact of magnetization on light polarization is well understood. Conversely, the manipulation of magnetism with polarized light is being investigated to achieve all-optical control of magnetism, driven by potential technological implementation in spintronics. Remarkable discoveries, such as the single-pulse all-optical switching of magnetization in thin films and submicrometer structures, have been reported. However, the demonstration of local optical control of magnetism at the nanoscale has remained elusive. Herein, it is demonstrated that exciting gold nanodiscs with circularly polarized femtosecond laser pulses lead to ultrafast, local, and deterministic control of magnetization in an adjacent magnetic film. This control is achieved by exploiting the magnetic moment generated in plasmonic nanodiscs through the inverse Faraday effect. The results pave the way for light-driven control in nanoscale spintronic devices and provide important insights into the generation of magnetic fields in plasmonic nanostructures. Ultrashort circularly polarized laser pulses are used to excite gold nanodiscs, activating localized plasmon resonance and generating strong magnetic field. The findings demonstrate that this magnetic field can effectively modulate the magnetization state of adjacent materials. These results pave the way for precise and deterministic control of magnetization at the nanoscale, presenting significant implications for future nanotechnology applications.image (c) 2024 WILEY-VCH GmbH

Place, publisher, year, edition, pages
John Wiley & Sons, 2025. Vol. 6, no 1
Keywords [en]
inverse Faraday effect, magnetization control, nanoplasmonics, ultrafast dynamics
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:uu:diva-555199DOI: 10.1002/adpr.202400083ISI: 001247897200001OAI: oai:DiVA.org:uu-555199DiVA, id: diva2:1954384
Available from: 2025-04-24 Created: 2025-04-24 Last updated: 2025-04-24Bibliographically approved

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Parchenko, SergiiHofhuis, KevinÅberg Larsson, AgneKapaklis, VassiliosScagnoli, ValerioHeyderman, Laura JaneKleibert, Armin
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