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Heat-conserving three-temperature model for ultrafast demagnetization in nickel
Department of Physics and Astronomy, Uppsala University, Sweden.ORCID iD: 0000-0002-5974-6160
Department of Physics and Astronomy, Uppsala University, Sweden.
Department of Physics and Astronomy, Uppsala University, Sweden ; School of Science and Technology, Örebro University, Sweden.ORCID iD: 0000-0001-8007-5392
Department of Physics and Astronomy, Uppsala University, Sweden.ORCID iD: 0000-0003-2977-255x
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2022 (English)In: Physical Review B, ISSN 2469-9950, E-ISSN 2469-9969, Vol. 106, no 17, article id 174407Article in journal (Refereed) Published
Abstract [en]

Multireservoir models are widely used for modeling and interpreting ultrafast magnetization dynamics. Here we introduce an alternative formulation to existing three-temperature models for the treatment of spin, electron, and lattice temperatures in magnetization dynamics simulations. In contrast to most existing models of calculations of energy transfer between reservoirs in these types of simulations, the heat distribution of the spin and lattice subsystems is evaluated during the simulation instead of being calculated a priori. The model is applied to investigate the demagnetization and remagnetization of fcc Ni, when subjected to a strong laser pulse. In particular, our model results in a fast interplay between the electron and spin subsystems which reproduces the main features of experimental data for fcc Ni significantly better than most reported three-temperature models. We also show that the way in which the electron, spin, and lattice heat capacities are described can have a significant impact on the simulated ultrafast dynamics. By introducing spin-lattice couplings in the simulation, it is shown that these explicit interactions only have a marginal impact on the magnetization dynamics of fcc Ni, albeit it is more pronounced for higher laser pulse powers.

Place, publisher, year, edition, pages
American Physical Society, 2022. Vol. 106, no 17, article id 174407
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:his:diva-24984DOI: 10.1103/PhysRevB.106.174407ISI: 000929827800003Scopus ID: 2-s2.0-85142310719OAI: oai:DiVA.org:his-24984DiVA, id: diva2:1949816
Funder
Knut and Alice Wallenberg Foundation, 2018.0060Swedish Research Council, 2019-03666Swedish Research Council, 2016-05980Swedish Research Council, 2019-05304Swedish Foundation for Strategic ResearchEU, European Research Council, 854843-FASTCORRStandUpSwedish Research Council, 2018-05973
Note

CC BY 4.0

This work was financially supported by the Knut and Alice Wallenberg Foundation through Grant No. 2018.0060. O.E. also acknowledges support by the Swedish Research Council (VR), the Foundation for Strategic Research (SSF), the European Research Council (Grant No. 854843-FASTCORR), and STandUP. O.E. and A.B. acknowledge eSSENCE. D.T. and A.D. acknowledge support from the Swedish Research Council (VR) through Grants No. 2019-03666, No. 2016-05980, and No. 2019-05304. The computations/data handling were/was enabled by resources provided by the Swedish National Infrastructure for Computing (SNIC), partially fundedby the Swedish Research Council through Grant Agreement No. 2018-05973.

Available from: 2025-04-03 Created: 2025-04-03 Last updated: 2025-05-07Bibliographically approved

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