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Inverse Uncertainty Quantification and Surrogate Models for Fuel Performance Modeling
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Applied Nuclear Physics.ORCID iD: 0000-0001-5296-7430
2025 (English)Doctoral thesis, comprehensive summary (Other academic)
Description
Abstract [en]

Nuclear power is a key electricity source, with light water reactors being the most common type. Their fuel typically consists of uranium dioxide pellets stacked in zirconium alloy cladding tubes. The purpose of the fuel is to produce heat and act as a barrier against releasing radioactive material. During operation, heat and radiation cause thermomechanical changes that can lead to fuel failure if not controlled. Thus, the nuclear industry needs efficient fuel performance codes with well-quantified uncertainties to predict fuel rod behavior. This thesis focuses on improving inverse uncertainty quantification and surrogate modeling for efficient fuel performance predictions.

Inverse uncertainty quantification is essential because fuel performance codes require calibrated model parameters to ensure that predictions match measurements. However, standard calibration methods often underestimate uncertainties due to unaccounted-for uncertainty sources, such as model inadequacy. Therefore, this thesis presents how unknown sources of uncertainty can be accounted for in calibration using Markov Chain Monte Carlo (MCMC) by assuming a variability in the calibration parameters. Two methods are presented, and both are based on MCMC, requiring numerous samples to converge. Hence, Gaussian Process (GP) surrogate modeling is used in place of the code to provide the calibration methods with inexpensive estimates of code responses. The first method is derivative-based, relying on differentiated GPs. While it effectively calibrates cladding oxidation, it struggles with fission gas release. Consequently, a more accurate method based on MH-within-Gibbs sampling is presented that successfully calibrates fission gas release.

The presented calibration methods use GP surrogate models to efficiently calibrate model parameters with inexpensive scalar estimates of code predictions. Beyond calibration, surrogate modeling is also essential when time-dependent predictions are needed for numerous fuel rod irradiations simultaneously. For example, if time-dependent predictions of fuel rod behavior are required in core optimization or core monitoring, calculation time can become a limiting factor. Therefore, this work also investigates neural network architectures for temporal data based on Temporal Convolutional Neural Networks (TCNs) and Fourier Neural Operators (FNOs) designed to model numerous fuel rods with varying irradiation histories. These networks accurately predict the behavior of thousands of fuel rods within seconds, significantly improving computational efficiency.

Place, publisher, year, edition, pages
Uppsala: Acta Universitatis Upsaliensis, 2025. , p. 110
Series
Digital Comprehensive Summaries of Uppsala Dissertations from the Faculty of Science and Technology, ISSN 1651-6214 ; 2522
Keywords [en]
Bayesian Calibration, Gaussian Process (GP), Markov Chain Monte Carlo (MCMC), TRANSURANUS, Temporal Frequency Network (TFN), Fourier Neural Operator (FNO), Temporal Convolutional Network (TCN), Fuel Performance Modeling, Surrogate Modeling, Inverse Uncertainty Quantification, Nuclear
National Category
Other Physics Topics
Research subject
Physics
Identifiers
URN: urn:nbn:se:uu:diva-553209ISBN: 978-91-513-2441-8 (print)OAI: oai:DiVA.org:uu-553209DiVA, id: diva2:1947075
Public defence
2025-05-16, Lecture hall Sonja Lyttkens, Ångströmlaboratoriet, Lägerhyddsvägen 1, Uppsala, 09:15 (English)
Opponent
Supervisors
Available from: 2025-04-22 Created: 2025-03-25 Last updated: 2025-04-22
List of papers
1. Treating model inadequacy in fuel performance model calibration by parameter uncertainty inflation
Open this publication in new window or tab >>Treating model inadequacy in fuel performance model calibration by parameter uncertainty inflation
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2022 (English)In: Annals of Nuclear Energy, ISSN 0306-4549, E-ISSN 1873-2100, Vol. 179, article id 109363Article in journal (Refereed) Published
Abstract [en]

The nuclear industry uses fuel performance codes to demonstrate integrity preservation of fuel rods. These codes include a complex system of models with empirical constants that one needs to calibrate for best estimates and uncertainties. However, deriving the appropriate level of uncertainty is often challenging due to model inadequacies.This paper presents a method to address model inadequacies by adapting the mean and covariance of the model parameters so that the propagated uncertainty conforms with the spread of the residuals rather than calibrating the model parameters directly.We demonstrate the method on synthetic data sets from an artificial test-bed containing a cladding oxidation and a hydrogen pick-up model. A repeated validation using many synthetic data sets shows that the method is robust and handles model inadequacies appropriately in most cases. Furthermore, we compare with traditional calibration and show model inadequacy leads to underestimation of uncertainties if not addressed.

Place, publisher, year, edition, pages
Elsevier, 2022
Keywords
Fuel performance modeling, Model inadequacy, Calibration, Bayesian, Markov Chain Monte Carlo, Inverse uncertainty quantification, Parameter uncertainty inflation
National Category
Energy Engineering
Identifiers
urn:nbn:se:uu:diva-486391 (URN)10.1016/j.anucene.2022.109363 (DOI)000858847800002 ()
Funder
Swedish Radiation Safety Authority
Available from: 2022-10-10 Created: 2022-10-10 Last updated: 2025-03-25Bibliographically approved
2. Surrogate Modeling with Derivative Prediction for Implementation in Inverse Uncertainty Quantification Methods for Fuel Performance Modeling
Open this publication in new window or tab >>Surrogate Modeling with Derivative Prediction for Implementation in Inverse Uncertainty Quantification Methods for Fuel Performance Modeling
2023 (English)In: TopFuel 2022 Light Water Reactor Fuel Performance Conference, American Nuclear Society, 2023, p. 375-381Conference paper, Published paper (Refereed)
Place, publisher, year, edition, pages
American Nuclear Society, 2023
National Category
Other Physics Topics
Identifiers
urn:nbn:se:uu:diva-500982 (URN)10.13182/TopFuel22-39392 (DOI)
Conference
TopFuel 2022 Light Water Reactor Fuel Performance Conference, Raleigh, NC, USA, 9-13 October, 2022
Available from: 2023-04-29 Created: 2023-04-29 Last updated: 2025-03-25Bibliographically approved
3. Model inadequacy in fuel performance code calibration: Derivative-based parameter uncertainty inflation
Open this publication in new window or tab >>Model inadequacy in fuel performance code calibration: Derivative-based parameter uncertainty inflation
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2024 (English)In: Annals of Nuclear Energy, ISSN 0306-4549, E-ISSN 1873-2100, Vol. 208, article id 110794Article in journal (Refereed) Published
Abstract [en]

Fuel performance codes are used to forecast fuel behavior and ensure safe operation. These analyses must typically include prediction uncertainties, and fuel performance models need calibration. Consequently, code calibration must derive the best estimates and corresponding uncertainties of model parameters for subsequent propagation.

Bayesian calibration is popular for generating the probability distribution of model parameters. However, model inadequacy disrupts these techniques, typically resulting in underestimated uncertainties. Earlier research showcased the incorporation of model inadequacy by model parameter inflation. The method demands cheap code predictions and derivatives, which required further research to develop differentiated Gaussian process surrogates.

This work combines those techniques into a complete methodology. We demonstrate it by calibrating Transuranus against fission gas release and cladding oxidation data. The result is model parameter uncertainties that primarily explain the discrepancies between the predictions and corresponding measurements, except when the output behaves highly non-linearly.

Place, publisher, year, edition, pages
Elsevier, 2024
Keywords
Calibration, Inverse uncertainty quantification, Fuel performance modeling, Fission gas release, Cladding oxidation, Model inadequacy, Transuranus code, Model parameter inflation
National Category
Subatomic Physics
Identifiers
urn:nbn:se:uu:diva-535332 (URN)10.1016/j.anucene.2024.110794 (DOI)001279475200001 ()
Funder
European CommissionSwedish Centre for Nuclear Technology (SKC)EU, European Research Council
Available from: 2024-07-25 Created: 2024-07-25 Last updated: 2025-03-25Bibliographically approved
4. Addressing Model Inadequacy In Fuel Performance Model Calibration Using Mh-Within-Gibbs Sampling
Open this publication in new window or tab >>Addressing Model Inadequacy In Fuel Performance Model Calibration Using Mh-Within-Gibbs Sampling
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2024 (English)Conference paper, Oral presentation with published abstract (Other academic)
Place, publisher, year, edition, pages
Nuclear and Industrial Engineering (NINE), 2024
National Category
Energy Engineering Subatomic Physics
Identifiers
urn:nbn:se:uu:diva-530505 (URN)
Conference
Best Estimate Plus Uncertainty International Conference (BEPU 2024), Real Collegio, Lucca, Tuscany, Italy, May 19–24, 2024
Available from: 2024-06-05 Created: 2024-06-05 Last updated: 2025-03-25Bibliographically approved
5. Addressing Model Inadequacies on CalibrationParameters in Fission Gas Release Modeling Using MH-within-Gibbs Sampling
Open this publication in new window or tab >>Addressing Model Inadequacies on CalibrationParameters in Fission Gas Release Modeling Using MH-within-Gibbs Sampling
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(English)Manuscript (preprint) (Other academic)
National Category
Other Physics Topics
Identifiers
urn:nbn:se:uu:diva-553191 (URN)
Available from: 2025-03-24 Created: 2025-03-24 Last updated: 2025-03-25
6. Deep heterogeneous joint architecture: A temporal frequency surrogate model for fuel codes
Open this publication in new window or tab >>Deep heterogeneous joint architecture: A temporal frequency surrogate model for fuel codes
2025 (English)In: Annals of Nuclear Energy, ISSN 0306-4549, E-ISSN 1873-2100, Vol. 211, article id 110893Article in journal (Refereed) Published
Abstract [en]

Fuel performance codes, such as Transuranus, predict fuel behavior and are used to ensure the safe operation of nuclear reactors. These codes are moderately time-consuming and affordable in many applications but may be limited in others, primarily when many fuel rods must be evaluated simultaneously. This work presents how the temporal neural network techniques, Temporal Convolutional Networks, and a Fourier Neural Operator can be combined to form a deep heterogeneous joint architecture as a surrogate model for fuel performance modeling in time-critical situations. We train the model using realistic power histories and corresponding outputs generated using the fuel performance code Transuranus. The ultimate result is a surrogate model for use in time-critical situations that take milliseconds to evaluate for thousands of fuel rods and have a mean test error of unseen data around a few percent.

Place, publisher, year, edition, pages
Elsevier, 2025
Keywords
Deep learning, Fuel performance modeling, Transuranus Code, TCN, FNO
National Category
Subatomic Physics
Identifiers
urn:nbn:se:uu:diva-538818 (URN)10.1016/j.anucene.2024.110893 (DOI)001306372300001 ()
Funder
Swedish Centre for Nuclear Technology (SKC)
Available from: 2024-10-02 Created: 2024-10-02 Last updated: 2025-03-25Bibliographically approved
7. A Time-Dependent Neural Network As A Surrogate For Fuel Performance Modeling
Open this publication in new window or tab >>A Time-Dependent Neural Network As A Surrogate For Fuel Performance Modeling
2024 (English)In: TopFuel 2024: Proceedings: Track 6: Modelling, analysis and methods, European Nuclear Society , 2024, p. 374-381Conference paper, Published paper (Refereed)
Place, publisher, year, edition, pages
European Nuclear Society, 2024
National Category
Physical Sciences
Identifiers
urn:nbn:se:uu:diva-546269 (URN)978-92-95064-41-6 (ISBN)
Conference
TopFuel 2024, Grenoble, France, 29 September - 3 October, 2024
Available from: 2025-01-08 Created: 2025-01-08 Last updated: 2025-03-25Bibliographically approved

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