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Dynamical Theory of Angle-Resolved Electron Energy Loss and Gain Spectroscopies of Phonons and Magnons in Transmission Electron Microscopy Including Multiple Scattering Effects
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory.ORCID iD: 0000-0002-4777-9993
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory.ORCID iD: 0000-0002-7018-244X
Uppsala University, Disciplinary Domain of Science and Technology, Physics, Department of Physics and Astronomy, Materials Theory.ORCID iD: 0000-0002-0074-1349
2025 (English)In: Physical Review Letters, ISSN 0031-9007, E-ISSN 1079-7114, Vol. 134, no 3, article id 036402Article in journal (Refereed) Published
Abstract [en]

We present a method for computing angle-resolved electron energy loss and gain spectroscopies for phonon and magnon excitations in transmission electron microscopy. Fractional scattering intensities are derived from the temperature-dependent time autocorrelation of the auxiliary electron beam wave function. This method captures both single and multiple scattering processes, as well as dynamical diffraction effects, while remaining computationally efficient and easy to parallelize.

Place, publisher, year, edition, pages
American Physical Society, 2025. Vol. 134, no 3, article id 036402
National Category
Condensed Matter Physics
Identifiers
URN: urn:nbn:se:uu:diva-551427DOI: 10.1103/PhysRevLett.134.036402ISI: 001415248700007PubMedID: 39927933Scopus ID: 2-s2.0-85215936374OAI: oai:DiVA.org:uu-551427DiVA, id: diva2:1940095
Part of project
Theory of modern spectroscopic methods at nanometer scale, Swedish Research Council
Funder
Swedish Research Council, 2022-06725Swedish Research Council, 2021-03848Knut and Alice Wallenberg Foundation, 2022.0079Olle Engkvists stiftelse, 214-0331The Swedish Foundation for International Cooperation in Research and Higher Education (STINT), CH2019-8211National Academic Infrastructure for Supercomputing in Sweden (NAISS)Available from: 2025-02-25 Created: 2025-02-25 Last updated: 2025-02-25Bibliographically approved

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