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Perspectives on Intermolecular Azomethine Ylide [3+2] Cycloadditions with Non-Electrophilic Olefins
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
Stockholm University, Faculty of Science, Department of Organic Chemistry.
2017 (English)In: Synthesis (Stuttgart), ISSN 0039-7881, E-ISSN 1437-210X, Vol. 49, no 4, p. 802-809Article, review/survey (Refereed) Published
Abstract [en]

Our interest in the synthesis of compact nitrogen heterocycles from abundant sources has motivated a critical analysis of the status in azomethine ylide chemistry. Despite the outstanding developments in catalytic enantioselective [3+2] cycloadditions, these are still limited to electron-poor olefins. Only a few examples can be found in the literature that report on cycloadditions using non-electrophilic alkenes and those are compiled herein. With this account we aim to extract lessons and challenges that will inspire future breakthroughs in this area.

Place, publisher, year, edition, pages
2017. Vol. 49, no 4, p. 802-809
Keywords [en]
heterocycles, pyrrolidines, anionic cycloaddition, azomethine ylide, catalysis
National Category
Chemical Sciences
Identifiers
URN: urn:nbn:se:su:diva-141374DOI: 10.1055/s-0036-1588662ISI: 000393233100012OAI: oai:DiVA.org:su-141374DiVA, id: diva2:1091982
Funder
Swedish Research CouncilVINNOVACarl Tryggers foundation Berzelii Centre EXSELENTAvailable from: 2017-04-28 Created: 2017-04-28 Last updated: 2018-03-02Bibliographically approved

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