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Two-dimensional charge transport in molecularly ordered polymer field-effect transistors
Ist Italian Tecnol, Italy; Politecn Milan, Italy.
Ist Italian Tecnol, Italy.
Linköping University, Department of Physics, Chemistry and Biology, Complex Materials and Devices. Linköping University, Faculty of Science & Engineering.
Linköping University, Department of Science and Technology, Physics and Electronics. Linköping University, Faculty of Science & Engineering. University of Groningen, Netherlands.ORCID iD: 0000-0001-7016-6514
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2016 (English)In: JOURNAL OF MATERIALS CHEMISTRY C, ISSN 2050-7526, Vol. 4, no 47, p. 11135-11142Article in journal (Refereed) Published
Abstract [en]

Nanometer-thick Langmuir-Schafer monolayers of an electron transporting polymer display charge transport, optical and electro-optical properties that do not depend on the number of layers deposited one above the other. This phenomenon can be rationalized with the micro-structure of the specific multi-layers, which introduces an interlayer hopping penalty confining transport to a neat 2D regime, with a channel not extending beyond a single similar to 3 nm thick polymer strand, as confirmed by kinetic Monte Carlo simulations. Such findings are critical to establish a quantitative structure-property nexus in high mobility polymer semiconductors and in the control of charge transport at a molecular scale.

Place, publisher, year, edition, pages
ROYAL SOC CHEMISTRY , 2016. Vol. 4, no 47, p. 11135-11142
National Category
Polymer Chemistry
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URN: urn:nbn:se:liu:diva-134079DOI: 10.1039/c6tc03897bISI: 000390725800016OAI: oai:DiVA.org:liu-134079DiVA, id: diva2:1068898
Note

Funding Agencies|European Research Council (ERC) under the European Unions Horizon research and innovation programme HEROIC [638059]; Knut och Alice Wallenbergs stiftelse; Advanced Functional Materials Center at Linkoping University [2009-00971]; VINNOVA [2015-04859]

Available from: 2017-01-26 Created: 2017-01-22 Last updated: 2017-02-17

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