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Combined Heterogeneous Metal/Chiral Amine: Multiple Relay Catalysis for Versatile Eco-Friendly Synthesis
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för organisk kemi.
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för organisk kemi.
Stockholms universitet, Naturvetenskapliga fakulteten, Institutionen för organisk kemi.
Vise andre og tillknytning
2014 (engelsk)Inngår i: Angewandte Chemie International Edition, ISSN 1433-7851, E-ISSN 1521-3773, Vol. 53, nr 13, s. 3447-3451Artikkel i tidsskrift (Fagfellevurdert) Published
Abstract [en]

Herein is described a versatile and broad synergistic strategy for expansion of chemical space and the synthesis of valuable molecules (e.g. carbocycles and heterocycles), with up to three quaternary stereocenters, in a highly enantioselective fashion from simple alcohols (31examples, 95:5 to >99.5:0.5 e.r.) using integrated heterogeneous metal/chiral amine multiple relay catalysis and air/O-2 as the terminal oxidant. A novel highly 1,4-selective heterogeneous metal/amine co-catalyzed hydrogenation of enals was also added to the relay catalysis sequences.

sted, utgiver, år, opplag, sider
2014. Vol. 53, nr 13, s. 3447-3451
Emneord [en]
alcohols, heterogeneous catalysis, homogeneous catalysis, hydrogenation, oxidation
HSV kategori
Identifikatorer
URN: urn:nbn:se:su:diva-102952DOI: 10.1002/anie.201310216ISI: 000333001500028OAI: oai:DiVA.org:su-102952DiVA, id: diva2:715019
Forskningsfinansiär
Swedish Research CouncilVINNOVAKnut and Alice Wallenberg Foundation
Merknad

AuthorCount:9;

Tilgjengelig fra: 2014-04-30 Laget: 2014-04-25 Sist oppdatert: 2017-12-05bibliografisk kontrollert

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